Abstract

Coupling of an atom-like emitter to surface plasmons provides a path toward significant optical non-linearity, which is essential in quantum information processing and quantum networks. A large coupling strength requires nanometer-scale positioning accuracy of the emitter near the surface of the plasmonic structure, which is challenging. We demonstrate the coupling of single localized defects in a tungsten diselenide (WSe2) monolayer self-aligned to the surface plasmon mode of a silver nanowire. The silver nanowire induces a strain gradient on the monolayer at the overlapping area, leading to the formation of localized defect emission sites that are intrinsically close to the surface plasmon. We measured an average coupling efficiency with a lower bound of 26% +/- 11% from the emitter into the plasmonic mode of the silver nanowire. This technique offers a way to achieve efficient coupling between plasmonic structures and localized defects of two-dimensional semiconductors.

Publication Details
Publication Type
Journal Article
Year of Publication
2017
Volume
17
Number of Pages
6564-6568
DOI
10.1021/acs.nanolett.7b02222
Journal
Nano Letters
Contributors