Abstract

Monolayer transition metal dichalcogenides (TMDs) host a variety of optically excited quasiparticle species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The magnetic response of these quasiparticles gives information on their spin and valley configurations, nuanced carrier interactions, and insight into the underlying band structure. Recently, there have been several reports of 2s/3s charged excitons in TMDs, but very little is still known about their response to external magnetic fields. Using photoluminescence excitation spectroscopy, we observe the presence of the 2s charged exciton and report its response to an applied magnetic field. We benchmark this response against the neutral exciton and find that both the 2s neutral and charged excitons exhibit similar behavior with g factors of gX2s0=−5.20±0.11 and gX2s−=−4.98±0.11, respectively.

Publication Details
Publication Type
Journal Article
Year of Publication
2022
Volume
106
Issue
8
Number of Pages
6
DOI
https://doi.org/10.1103/PhysRevB.106.L081409
URL
https://journals.aps.org/prb/abstract/10.1103/PhysRevB.106.L081409
Journal
Phys. Rev. B
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Contributors
Start Page
L081409
Date Published
08/2022