Abstract

Optical excitations in moiré transition metal dichalcogenide bilayers lead to the creation of excitons, as electron-hole bound states, that are generically considered within a Bose-Hubbard framework. Here, we demonstrate that these composite particles obey an angular momentum commutation relation that is generally nonbosonic. This emergent spin description of excitons indicates a limitation to their occupancy on each site, which is substantial in the weak electron-hole binding regime. The effective exciton theory is accordingly a spin Hamiltonian, which further becomes a Hubbard model of emergent bosons subject to an occupancy constraint after a Holstein-Primakoff transformation. We apply our theory to three commonly studied bilayers (MoSe2/WSe2, WSe2/WS2, and WSe2/MoS2) and show that in the relevant parameter regimes their allowed occupancies never exceed three excitons. Our systematic theory provides guidelines for future research on the many-body physics of moiré excitons.

Publication Details
Publication Type
Journal Article
Year of Publication
2024
Volume
132
Issue
186202
DOI
10.1103/PhysRevLett.132.186202
URL
https://journals.aps.org/prl/abstract/10.1103/PhysRevLett.132.186202
Journal
Physical Review Letters
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Date Published
04/2024